Vapour–liquid–solid growth of monolayer MoS2 nanoribbons View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-06

AUTHORS

Shisheng Li, Yung-Chang Lin, Wen Zhao, Jing Wu, Zhuo Wang, Zehua Hu, Youde Shen, Dai-Ming Tang, Junyong Wang, Qi Zhang, Hai Zhu, Leiqiang Chu, Weijie Zhao, Chang Liu, Zhipei Sun, Takaaki Taniguchi, Minoru Osada, Wei Chen, Qing-Hua Xu, Andrew Thye Shen Wee, Kazu Suenaga, Feng Ding, Goki Eda

ABSTRACT

Chemical vapour deposition of two-dimensional materials typically involves the conversion of vapour precursors to solid products in a vapour-solid-solid mode. Here, we report the vapour-liquid-solid growth of monolayer MoS2, yielding highly crystalline ribbons with a width of few tens to thousands of nanometres. This vapour-liquid-solid growth is triggered by the reaction between MoO3 and NaCl, which results in the formation of molten Na-Mo-O droplets. These droplets mediate the growth of MoS2 ribbons in the 'crawling mode' when saturated with sulfur. The locally well-defined orientations of the ribbons reveal the regular horizontal motion of the droplets during growth. Using atomic-resolution scanning transmission electron microscopy and second harmonic generation microscopy, we show that the ribbons are grown homoepitaxially on monolayer MoS2 with predominantly 2H- or 3R-type stacking. Our findings highlight the prospects for the controlled growth of atomically thin nanostructure arrays for nanoelectronic devices and the development of unique mixed-dimensional structures. More... »

PAGES

535-542

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41563-018-0055-z

DOI

http://dx.doi.org/10.1038/s41563-018-0055-z

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1103549260

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29686277


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