Cold quantum-controlled rotationally inelastic scattering of HD with H2 and D2 reveals collisional partner reorientation View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-05

AUTHORS

William E. Perreault, Nandini Mukherjee, Richard N. Zare

ABSTRACT

Molecular interactions are best probed by scattering experiments. Interpretation of these studies has been limited by lack of control over the quantum states of the incoming collision partners. We report here the rotationally inelastic collisions of quantum-state prepared deuterium hydride (HD) with H2 and D2 using a method that provides an improved control over the input states. HD was coexpanded with its partner in a single supersonic beam, which reduced the collision temperature to 0-5 K, and thereby restricted the involved incoming partial waves to s and p. By preparing HD with its bond axis preferentially aligned parallel and perpendicular to the relative velocity of the colliding partners, we observed that the rotational relaxation of HD depends strongly on the initial bond-axis orientation. We developed a partial-wave analysis that conclusively demonstrates that the scattering mechanism involves the exchange of internal angular momentum between the colliding partners. The striking differences between H2/HD and D2/HD scattering suggest the presence of anisotropically sensitive resonances. More... »

PAGES

561-567

Journal

TITLE

Nature Chemistry

ISSUE

5

VOLUME

10

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41557-018-0028-5

DOI

http://dx.doi.org/10.1038/s41557-018-0028-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1103276913

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29662208


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