Spin liquid and ferroelectricity close to a quantum critical point in PbCuTe2O6 View Full Text


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Article Info

DATE

2021-11-19

AUTHORS

Christian Thurn, Paul Eibisch, Arif Ata, Maximilian Winkler, Peter Lunkenheimer, István Kézsmárki, Ulrich Tutsch, Yohei Saito, Steffi Hartmann, Jan Zimmermann, Abanoub R. N. Hanna, A. T. M. Nazmul Islam, Shravani Chillal, Bella Lake, Bernd Wolf, Michael Lang

ABSTRACT

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favor of more exotic states such as spin liquids. By following this guiding principle, a number of spin liquid candidate systems were identified in quasi-two-dimensional (quasi-2D) systems. For 3D, however, the situation is less favorable as quantum fluctuations are reduced and competing states become more relevant. Here we report a comprehensive study of thermodynamic, magnetic and dielectric properties on single crystalline and pressed-powder samples of PbCuTe2O6, a candidate material for a 3D frustrated quantum spin liquid featuring a hyperkagome lattice. Whereas the low-temperature properties of the powder samples are consistent with the recently proposed quantum spin liquid state, an even more exotic behavior is revealed for the single crystals. These crystals show ferroelectric order at TFE ≈ 1 K, accompanied by strong lattice distortions, and a modified magnetic response—still consistent with a quantum spin liquid—but with clear indications for quantum critical behavior. More... »

PAGES

95

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41535-021-00395-6

DOI

http://dx.doi.org/10.1038/s41535-021-00395-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1142685251


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34 favor
35 ferroelectric order
36 ferroelectricity
37 fluctuations
38 frustration
39 geometrical frustration
40 hyperkagome lattice
41 indications
42 lattice
43 lattice distortion
44 liquid
45 liquid state
46 long-range magnetic order
47 low-temperature properties
48 magnetic order
49 magnetic response
50 materials
51 number
52 order
53 point
54 powder samples
55 principles
56 properties
57 quantum critical behavior
58 quantum critical point
59 quantum fluctuations
60 quantum spin liquid
61 quantum spin liquid state
62 response
63 samples
64 single crystalline
65 single crystals
66 situation
67 spin
68 spin liquid
69 spin liquid state
70 state
71 strong lattice distortion
72 strong quantum fluctuations
73 study
74 system
75 thermodynamics
76 two-dimensional systems
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