Connection between Mott physics and crystal structure in a series of transition metal binary compounds View Full Text


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Article Info

DATE

2019-12

AUTHORS

Nicola Lanatà, Tsung-Han Lee, Yong-Xin Yao, Vladan Stevanović, Vladimir Dobrosavljević

ABSTRACT

The choice that a solid system “makes” when adopting a crystal structure (stable or metastable) is ultimately governed by the interactions between electrons forming chemical bonds. Here we analyze six prototypical binary transition metal compounds and shed light on the connection between Mott physics and the behavior of the energy as a function of the spatial arrangement of the atoms in these systems. Remarkably, we find that the main qualitative features of this complex behavior in the Mott phase of these systems can be traced back to the fact that the strong d-electron correlations influence substantially the charge transfer mechanism, which, in turn, controls the electrostatic interactions. This result advances our understanding of the influence of strong correlations on the crystal structure, opens a new avenue for extending structure prediction methodologies to strongly correlated materials, and paves the way for predicting and studying metastability and polymorphism in these systems. More... »

PAGES

30

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41524-019-0169-0

DOI

http://dx.doi.org/10.1038/s41524-019-0169-0

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112543898


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