Compositional dependence of the fragility in metallic glass forming liquids View Full Text


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Article Info

DATE

2022-06-28

AUTHORS

Sebastian A. Kube, Sungwoo Sohn, Rodrigo Ojeda-Mota, Theo Evers, William Polsky, Naijia Liu, Kevin Ryan, Sean Rinehart, Yong Sun, Jan Schroers

ABSTRACT

The viscosity and its temperature dependence, the fragility, are key properties of a liquid. A low fragility is believed to promote the formation of metallic glasses. Yet, the fragility remains poorly understood, since experimental data of its compositional dependence are scarce. Here, we introduce the film inflation method (FIM), which measures the fragility of metallic glass forming liquids across wide ranges of composition and glass-forming ability. We determine the fragility for 170 alloys ranging over 25 at.% in Mg–Cu–Y. Within this alloy system, large fragility variations are observed. Contrary to the general understanding, a low fragility does not correlate with high glass-forming ability here. We introduce crystallization complexity as an additional contribution, which can potentially become significant when modeling glass forming ability over many orders of magnitude. More... »

PAGES

3708

References to SciGraph publications

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  • 2006-09. Improving glass-forming ability of Mg−Cu−Y via substitutional alloying: Effects of Ag versus Ni in JOURNAL OF MATERIALS RESEARCH
  • 2019-05-09. Formation and stability of complex metallic phases including quasicrystals explored through combinatorial methods in SCIENTIFIC REPORTS
  • 1993-12. Confusion by design in NATURE
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  • 2015-05-20. New horizons for glass formation and stability in NATURE MATERIALS
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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41467-022-31314-3

    DOI

    http://dx.doi.org/10.1038/s41467-022-31314-3

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1149021667

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/35764635


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