Quantum spins and hybridization in artificially-constructed chains of magnetic adatoms on a superconductor View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2022-04-20

AUTHORS

Eva Liebhaber, Lisa M. Rütten, Gaël Reecht, Jacob F. Steiner, Sebastian Rohlf, Kai Rossnagel, Felix von Oppen, Katharina J. Franke

ABSTRACT

Magnetic adatom chains on surfaces constitute fascinating quantum spin systems. Superconducting substrates suppress interactions with bulk electronic excitations but couple the adatom spins to a chain of subgap Yu-Shiba-Rusinov (YSR) quasiparticles. Using a scanning tunneling microscope, we investigate such correlated spin-fermion systems by constructing Fe chains adatom by adatom on superconducting NbSe2. The adatoms couple entirely via the substrate, retaining their quantum spin nature. In dimers, we observe that the deepest YSR state undergoes a quantum phase transition due to Ruderman-Kittel-Kasuya-Yosida interactions, a distinct signature of quantum spins. Chains exhibit coherent hybridization and band formation of the YSR excitations, indicating ferromagnetic coupling. Longer chains develop separate domains due to coexisting charge-density-wave order of NbSe2. Despite the spin-orbit-coupled substrate, we find no signatures of Majoranas, possibly because quantum spins reduce the parameter range for topological superconductivity. We suggest that adatom chains are versatile systems for investigating correlated-electron physics and its interplay with topological superconductivity. More... »

PAGES

2160

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-022-29879-0

DOI

http://dx.doi.org/10.1038/s41467-022-29879-0

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1147253567

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/35443753


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