Large-gap insulating dimer ground state in monolayer IrTe2 View Full Text


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Article Info

DATE

2022-02-16

AUTHORS

Jinwoong Hwang, Kyoo Kim, Canxun Zhang, Tiancong Zhu, Charlotte Herbig, Sooran Kim, Bongjae Kim, Yong Zhong, Mohamed Salah, Mohamed M. El-Desoky, Choongyu Hwang, Zhi-Xun Shen, Michael F. Crommie, Sung-Kwan Mo

ABSTRACT

Monolayers of two-dimensional van der Waals materials exhibit novel electronic phases distinct from their bulk due to the symmetry breaking and reduced screening in the absence of the interlayer coupling. In this work, we combine angle-resolved photoemission spectroscopy and scanning tunneling microscopy/spectroscopy to demonstrate the emergence of a unique insulating 2 × 1 dimer ground state in monolayer 1T-IrTe2 that has a large band gap in contrast to the metallic bilayer-to-bulk forms of this material. First-principles calculations reveal that phonon and charge instabilities as well as local bond formation collectively enhance and stabilize a charge-ordered ground state. Our findings provide important insights into the subtle balance of interactions having similar energy scales that occurs in the absence of strong interlayer coupling, which offers new opportunities to engineer the properties of 2D monolayers. More... »

PAGES

906

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-022-28542-y

DOI

http://dx.doi.org/10.1038/s41467-022-28542-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1145604321

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/35173153


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