Boson-peak-like anomaly caused by transverse phonon softening in strain glass View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2021-10-01

AUTHORS

Shuai Ren, Hong-Xiang Zong, Xue-Fei Tao, Yong-Hao Sun, Bao-An Sun, De-Zhen Xue, Xiang-Dong Ding, Wei-Hua Wang

ABSTRACT

Strain glass is a glassy state with frozen ferroelastic/martensitic nanodomains in shape memory alloys, yet its nature remains unclear. Here, we report a glassy feature in strain glass that was thought to be only present in structural glasses. An abnormal hump is observed in strain glass around 10 K upon normalizing the specific heat by cubed temperature, similar to the boson peak in metallic glass. The simulation studies show that this boson-peak-like anomaly is caused by the phonon softening of the non-transforming matrix surrounding martensitic domains, which occurs in a transverse acoustic branch not associated with the martensitic transformation displacements. Therefore, this anomaly neither is a relic of van Hove singularity nor can be explained by other theories relying on structural disorder, while it verifies a recent theoretical model without any assumptions of disorder. This work might provide fresh insights in understanding the nature of glassy states and associated vibrational properties. More... »

PAGES

5755

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-021-26029-w

DOI

http://dx.doi.org/10.1038/s41467-021-26029-w

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1141548020

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/34599172


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