Decoupling between calorimetric and dynamical glass transitions in high-entropy metallic glasses View Full Text


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Article Info

DATE

2021-06-22

AUTHORS

Jing Jiang, Zhen Lu, Jie Shen, Takeshi Wada, Hidemi Kato, Mingwei Chen

ABSTRACT

Glass transition is one of the unresolved critical issues in solid-state physics and materials science, during which a viscous liquid is frozen into a solid or structurally arrested state. On account of the uniform arrested mechanism, the calorimetric glass transition temperature (Tg) always follows the same trend as the dynamical glass transition (or α-relaxation) temperature (Tα) determined by dynamic mechanical analysis (DMA). Here, we explored the correlations between the calorimetric and dynamical glass transitions of three prototypical high-entropy metallic glasses (HEMGs) systems. We found that the HEMGs present a depressed dynamical glass transition phenomenon, i.e., HEMGs with moderate calorimetric Tg represent the highest Tα and the maximum activation energy of α-relaxation. These decoupled glass transitions from thermal and mechanical measurements reveal the effect of high configurational entropy on the structure and dynamics of supercooled liquids and metallic glasses, which are associated with sluggish diffusion and decreased dynamic and spatial heterogeneities from high mixing entropy. The results have important implications in understanding the entropy effect on the structure and properties of metallic glasses for designing new materials with plenteous physical and mechanical performances. More... »

PAGES

3843

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-021-24093-w

DOI

http://dx.doi.org/10.1038/s41467-021-24093-w

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https://app.dimensions.ai/details/publication/pub.1139036082

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/34158476


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