IrW nanochannel support enabling ultrastable electrocatalytic oxygen evolution at 2 A cm−2 in acidic media View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2021-06-10

AUTHORS

Rui Li, Haiyun Wang, Fei Hu, K. C. Chan, Xiongjun Liu, Zhaoping Lu, Jing Wang, Zhibin Li, Longjiao Zeng, Yuanyuan Li, Xiaojun Wu, Yujie Xiong

ABSTRACT

A grand challenge for proton exchange membrane electrolyzers is the rational design of oxygen evolution reaction electrocatalysts to balance activity and stability. Here, we report a support-stabilized catalyst, the activated ~200 nm-depth IrW nanochannel that achieves the current density of 2 A cm−2 at an overpotential of only ~497 mV and maintains ultrastable gas evolution at 100 mA cm−2 at least 800 h with a negligible degradation rate of ~4 μV h−1. Structure analyses combined with theoretical calculations indicate that the IrW support alters the charge distribution of surface (IrO2)n clusters and effectively confines the cluster size within 4 (n≤4). Such support-stabilizing effect prevents the surface Ir from agglomeration and retains a thin layer of electrocatalytically active IrO2 clusters on surface, realizing a win-win strategy for ultrahigh OER activity and stability. This work would open up an opportunity for engineering suitable catalysts for robust proton exchange membrane-based electrolyzers. More... »

PAGES

3540

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-021-23907-1

DOI

http://dx.doi.org/10.1038/s41467-021-23907-1

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1138766442

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/34112770


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