Selective photoelectrochemical oxidation of glycerol to high value-added dihydroxyacetone View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-04-16

AUTHORS

Dong Liu, Jin-Cheng Liu, Weizheng Cai, Jun Ma, Hong Bin Yang, Hai Xiao, Jun Li, Yujie Xiong, Yanqiang Huang, Bin Liu

ABSTRACT

It is highly profitable to transform glycerol – the main by-product from biodiesel production to high value-added chemicals. In this work, we develop a photoelectrochemical system based on nanoporous BiVO4 for selective oxidation of glycerol to 1,3-dihydroxyacetone – one of the most valuable derivatives of glycerol. Under AM 1.5G front illumination (100 mW cm−2) in an acidic medium (pH = 2) without adscititious oxidant, the nanoporous BiVO4 photoanode achieves a glycerol oxidation photocurrent density of 3.7 mA cm−2 at a potential of 1.2 V versus RHE with 51% 1,3-dihydroxyacetone selectivity, equivalent to a production rate of 200 mmol of 1,3-dihydroxyacetone per m2 of illumination area in one hour. More... »

PAGES

1779

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-09788-5

DOI

http://dx.doi.org/10.1038/s41467-019-09788-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113481179

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30992441


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