Boosting the efficiency of organic persistent room-temperature phosphorescence by intramolecular triplet-triplet energy transfer. View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Weijun Zhao, Tsz Shing Cheung, Nan Jiang, Wenbin Huang, Jacky W Y Lam, Xuepeng Zhang, Zikai He, Ben Zhong Tang

ABSTRACT

Persistent luminescence is a fascinating phenomenon with exceptional applications. However, the development of organic materials capable of persistent luminescence, such as organic persistent room-temperature phosphorescence, lags behind for their normally low efficiency. Moreover, enhancing the phosphorescence efficiency of organic luminophores often results in short lifetime, which sets an irreconcilable obstacle. Here we report a strategy to boost the efficiency of phosphorescence by intramolecular triplet-triplet energy transfer. Incorpotation of (bromo)dibenzofuran or (bromo)dibenzothiophene to carbazole has boosted the intersystem crossing and provided an intramolecular triplet-state bridge to offer a near quantitative exothermic triplet-triplet energy transfer to repopulate the lowest triplet-state of carbazole. All these factors work together to contribute the efficient phosphorescence. The generation and transfer of triplet excitons within a single molecule is revealed by low-temperature spectra, energy level and lifetime investigations. The strategy developed here will enable the development of efficient phosphorescent materials for potential high-tech applications. More... »

PAGES

1595

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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41467-019-09561-8

    DOI

    http://dx.doi.org/10.1038/s41467-019-09561-8

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1113300673

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/30962451


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