Anion-adaptive crystalline cationic material for 99TcO4- trapping. View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Lei Mei, Fei-Ze Li, Jian-Hui Lan, Cong-Zhi Wang, Chao Xu, Hao Deng, Qun-Yan Wu, Kong-Qiu Hu, Lin Wang, Zhi-Fang Chai, Jing Chen, John K Gibson, Wei-Qun Shi

ABSTRACT

Efficient anion recognition is of great significance for radioactive 99TcO4- decontamination, but it remains a challenge for traditional sorbents. Herein, we put forward a tactic using soft crystalline cationic material with anion-adaptive dynamics for 99TcO4- sequestration. A cucurbit[8]uril-based supramolecular metal-organic material is produced through a multi-component assembly strategy and used as a sorbent for effective trapping of TcO4-. Excellent separation of TcO4-/ReO4- is demonstrated by fast removal kinetics, good sorption capacity and high distribution coefficient. Remarkably, the most superior selectivity among metal-organic materials reported so far, together with good hydrolytic stability, indicates potential for efficient TcO4- removal. The structure incorporating ReO4- reveals that the supramolecular framework undergoes adaptive reconstruction facilitating the effective accommodation of TcO4-/ReO4-. The results highlight opportunities for development of soft anion-adaptive sorbents for highly selective anion decontamination. More... »

PAGES

1532

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-09504-3

DOI

http://dx.doi.org/10.1038/s41467-019-09504-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113184991

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30948745


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