Design of next-generation ceramic fuel cells and real-time characterization with synchrotron X-ray diffraction computed tomography View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Tao Li, Thomas M. M. Heenan, Mohamad F. Rabuni, Bo Wang, Nicholas M. Farandos, Geoff H. Kelsall, Dorota Matras, Chun Tan, Xuekun Lu, Simon D. M. Jacques, Dan J. L. Brett, Paul R. Shearing, Marco Di Michiel, Andrew M. Beale, Antonis Vamvakeros, Kang Li

ABSTRACT

Ceramic fuel cells offer a clean and efficient means of producing electricity through a variety of fuels. However, miniaturization of cell dimensions for portable device application remains a challenge, as volumetric power densities generated by readily-available planar/tubular ceramic cells are limited. Here, we demonstrate a concept of 'micro-monolithic' ceramic cell design. The mechanical robustness and structural integrity of this design is thoroughly investigated with real-time, synchrotron X-ray diffraction computed tomography, suggesting excellent thermal cycling stability. The successful miniaturization results in an exceptional power density of 1.27 W cm-2 at 800 °C, which is among the highest reported. This holistic design incorporates both mechanical integrity and electrochemical performance, leading to mechanical property enhancement and representing an important step toward commercial development of portable ceramic devices with high volumetric power (>10 W cm-3), fast thermal cycling and marked mechanical reliability. More... »

PAGES

1497

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-09427-z

DOI

http://dx.doi.org/10.1038/s41467-019-09427-z

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113170115

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30940801


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