Urban pollution greatly enhances formation of natural aerosols over the Amazon rainforest View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Manish Shrivastava, Meinrat O. Andreae, Paulo Artaxo, Henrique M. J. Barbosa, Larry K. Berg, Joel Brito, Joseph Ching, Richard C. Easter, Jiwen Fan, Jerome D. Fast, Zhe Feng, Jose D. Fuentes, Marianne Glasius, Allen H. Goldstein, Eliane Gomes Alves, Helber Gomes, Dasa Gu, Alex Guenther, Shantanu H. Jathar, Saewung Kim, Ying Liu, Sijia Lou, Scot T. Martin, V. Faye McNeill, Adan Medeiros, Suzane S. de Sá, John E. Shilling, Stephen R. Springston, R. A. F. Souza, Joel A. Thornton, Gabriel Isaacman-VanWertz, Lindsay D. Yee, Rita Ynoue, Rahul A. Zaveri, Alla Zelenyuk, Chun Zhao

ABSTRACT

One of the least understood aspects in atmospheric chemistry is how urban emissions influence the formation of natural organic aerosols, which affect Earth's energy budget. The Amazon rainforest, during its wet season, is one of the few remaining places on Earth where atmospheric chemistry transitions between preindustrial and urban-influenced conditions. Here, we integrate insights from several laboratory measurements and simulate the formation of secondary organic aerosols (SOA) in the Amazon using a high-resolution chemical transport model. Simulations show that emissions of nitrogen-oxides from Manaus, a city of ~2 million people, greatly enhance production of biogenic SOA by 60-200% on average with peak enhancements of 400%, through the increased oxidation of gas-phase organic carbon emitted by the forests. Simulated enhancements agree with aircraft measurements, and are much larger than those reported over other locations. The implication is that increasing anthropogenic emissions in the future might substantially enhance biogenic SOA in pristine locations like the Amazon. More... »

PAGES

1046

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-08909-4

DOI

http://dx.doi.org/10.1038/s41467-019-08909-4

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112543877

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30837467


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100 schema:description One of the least understood aspects in atmospheric chemistry is how urban emissions influence the formation of natural organic aerosols, which affect Earth's energy budget. The Amazon rainforest, during its wet season, is one of the few remaining places on Earth where atmospheric chemistry transitions between preindustrial and urban-influenced conditions. Here, we integrate insights from several laboratory measurements and simulate the formation of secondary organic aerosols (SOA) in the Amazon using a high-resolution chemical transport model. Simulations show that emissions of nitrogen-oxides from Manaus, a city of ~2 million people, greatly enhance production of biogenic SOA by 60-200% on average with peak enhancements of 400%, through the increased oxidation of gas-phase organic carbon emitted by the forests. Simulated enhancements agree with aircraft measurements, and are much larger than those reported over other locations. The implication is that increasing anthropogenic emissions in the future might substantially enhance biogenic SOA in pristine locations like the Amazon.
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