Composition change-driven texturing and doping in solution-processed SnSe thermoelectric thin films View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Seung Hwae Heo, Seungki Jo, Hyo Seok Kim, Garam Choi, Jae Yong Song, Jun-Yun Kang, No-Jin Park, Hyeong Woo Ban, Fredrick Kim, Hyewon Jeong, Jaemin Jung, Jaeyoung Jang, Won Bo Lee, Hosun Shin, Jae Sung Son

ABSTRACT

The discovery of SnSe single crystals with record high thermoelectric efficiency along the b-axis has led to the search for ways to synthesize polycrystalline SnSe with similar efficiencies. However, due to weak texturing and difficulties in doping, such high thermoelectric efficiencies have not been realized in polycrystals or thin films. Here, we show that highly textured and hole doped SnSe thin films with thermoelectric power factors at the single crystal level can be prepared by solution process. Purification step in the synthetic process produced a SnSe-based chalcogenidometallate precursor, which decomposes to form the SnSe2 phase. We show that the strong textures of the thin films in the b-c plane originate from the transition of two dimensional SnSe2 to SnSe. This composition change-driven transition offers wide control over composition and doping of the thin films. Our optimum SnSe thin films exhibit a thermoelectric power factor of 4.27 μW cm-1 K-2. More... »

PAGES

864

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-08883-x

DOI

http://dx.doi.org/10.1038/s41467-019-08883-x

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112228204

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30787291


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