Disorder in Mn+1AXn phases at the atomic scale View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Chenxu Wang, Tengfei Yang, Cameron L. Tracy, Chenyang Lu, Hui Zhang, Yong-Jie Hu, Lumin Wang, Liang Qi, Lin Gu, Qing Huang, Jie Zhang, Jingyang Wang, Jianming Xue, Rodney C. Ewing, Yugang Wang

ABSTRACT

Atomic disordering in materials alters their physical and chemical properties and can subsequently affect their performance. In complex ceramic materials, it is a challenge to understand the nature of structural disordering, due to the difficulty of direct, atomic-scale experimental observations. Here we report the direct imaging of ion irradiation-induced antisite defects in Mn+1AXn phases using double CS-corrected scanning transmission electron microscopy and provide compelling evidence of order-to-disorder phase transformations, overturning the conventional view that irradiation causes phase decomposition to binary fcc-structured Mn+1Xn. With the formation of uniformly distributed cation antisite defects and the rearrangement of X anions, disordered solid solution γ-(Mn+1A)Xn phases are formed at low ion fluences, followed by gradual transitions to solid solution fcc-structured (Mn+1A)Xn phases. This study provides a comprehensive understanding of the order-to-disorder transformations in Mn+1AXn phases and proposes a method for the synthesis of new solid solution (Mn+1A)Xn phases by tailoring the disorder. More... »

PAGES

622

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-08588-1

DOI

http://dx.doi.org/10.1038/s41467-019-08588-1

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111980313

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30733461


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