Ultrafast hole transfer mediated by polaron pairs in all-polymer photovoltaic blends View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Rui Wang, Yao Yao, Chunfeng Zhang, Yindong Zhang, Haijun Bin, Lingwei Xue, Zhi-Guo Zhang, Xiaoyu Xie, Haibo Ma, Xiaoyong Wang, Yongfang Li, Min Xiao

ABSTRACT

The charge separation yield at a bulk heterojunction sets the upper efficiency limit of an organic solar cell. Ultrafast charge transfer processes in polymer/fullerene blends have been intensively studied but much less is known about these processes in all-polymer systems. Here, we show that interfacial charge separation can occur through a polaron pair-derived hole transfer process in all-polymer photovoltaic blends, which is a fundamentally different mechanism compared to the exciton-dominated pathway in the polymer/fullerene blends. By utilizing ultrafast optical measurements, we have clearly identified an ultrafast hole transfer process with a lifetime of about 3 ps mediated by photo-excited polaron pairs which has a markedly high quantum efficiency of about 97%. Spectroscopic data show that excitons act as spectators during the efficient hole transfer process. Our findings suggest an alternative route to improve the efficiency of all-polymer solar devices by manipulating polaron pairs. More... »

PAGES

398

References to SciGraph publications

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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41467-019-08361-4

    DOI

    http://dx.doi.org/10.1038/s41467-019-08361-4

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1111630978

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/30674887


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