Photoinduced semiconductor-metal transition in ultrathin troilite FeS nanosheets to trigger efficient hydrogen evolution View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Gang Zhou, Yun Shan, Longlu Wang, Youyou Hu, Junhong Guo, Fangren Hu, Jiancang Shen, Yu Gu, Jingteng Cui, Lizhe Liu, Xinglong Wu

ABSTRACT

The exploitation of the stable and earth-abundant electrocatalyst with high catalytic activity remains a significant challenge for hydrogen evolution reaction. Being different from complex nanostructuring, this work focuses on a simple and feasible way to improve hydrogen evolution reaction performance via manipulation of intrinsic physical properties of the material. Herein, we present an interesting semiconductor-metal transition in ultrathin troilite FeS nanosheets triggered by near infrared radiation at near room temperature for the first time. The photogenerated metal-phase FeS nanosheets demonstrate intrinsically high catalytic activity and fast carrier transfer for hydrogen evolution reaction, leading to an overpotential of 142 mV at 10 mA cm-2 and a lower Tafel slope of 36.9 mV per decade. Our findings provide new inspirations for the steering of electron transfer and designing new-type catalysts. More... »

PAGES

399

References to SciGraph publications

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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41467-019-08358-z

    DOI

    http://dx.doi.org/10.1038/s41467-019-08358-z

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1111633267

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/30674896


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    279 Key Laboratory of Modern Acoustics, MOE, Institute of Acoustics and Collaborative Innovation Center of Advanced Microstructures, National Laboratory of Solid State Microstructures, Nanjing University, 210093, Nanjing, People’s Republic of China
    280 rdf:type schema:Organization
    281 https://www.grid.ac/institutes/grid.453246.2 schema:alternateName Nanjing University of Posts and Telecommunications
    282 schema:name School of Optoelectronic Engineering and Grüenberg Research Centre, Nanjing University of Posts and Telecommunications, 210023, Nanjing, People’s Republic of China
    283 rdf:type schema:Organization
    284 https://www.grid.ac/institutes/grid.67293.39 schema:alternateName Hunan University
    285 schema:name School of Physics and Electronics, Hunan University, 410082, Changsha, People’s Republic of China
    286 rdf:type schema:Organization
     




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