Most Earth-surface calcites precipitate out of isotopic equilibrium View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

M. Daëron, R. N. Drysdale, M. Peral, D. Huyghe, D. Blamart, T. B. Coplen, F. Lartaud, G. Zanchetta

ABSTRACT

Oxygen-isotope thermometry played a critical role in the rise of modern geochemistry and remains extensively used in (bio-)geoscience. Its theoretical foundations rest on the assumption that 18O/16O partitioning among water and carbonate minerals primarily reflects thermodynamic equilibrium. However, after decades of research, there is no consensus on the true equilibrium 18O/16O fractionation between calcite and water (18αcc/w). Here, we constrain the equilibrium relations linking temperature, 18αcc/w, and clumped isotopes (Δ47) based on the composition of extremely slow-growing calcites from Devils Hole and Laghetto Basso (Corchia Cave). Equilibrium 18αcc/w values are systematically ~1.5‰ greater than those in biogenic and synthetic calcite traditionally considered to approach oxygen-isotope equilibrium. We further demonstrate that subtle disequilibria also affect Δ47 in biogenic calcite. These observations provide evidence that most Earth-surface calcites fail to achieve isotopic equilibrium, highlighting the need to improve our quantitative understanding of non-equilibrium isotope fractionation effects instead of relying on phenomenological calibrations. More... »

PAGES

429

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-019-08336-5

DOI

http://dx.doi.org/10.1038/s41467-019-08336-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111656728

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30683869


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