Lithium intercalation into bilayer graphene View Full Text


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Article Info

DATE

2019-01-17

AUTHORS

Kemeng Ji, Jiuhui Han, Akihiko Hirata, Takeshi Fujita, Yuhao Shen, Shoucong Ning, Pan Liu, Hamzeh Kashani, Yuan Tian, Yoshikazu Ito, Jun-ichi Fujita, Yutaka Oyama

ABSTRACT

The real capacity of graphene and the lithium-storage process in graphite are two currently perplexing problems in the field of lithium ion batteries. Here we demonstrate a three-dimensional bilayer graphene foam with few defects and a predominant Bernal stacking configuration, and systematically investigate its lithium-storage capacity, process, kinetics, and resistances. We clarify that lithium atoms can be stored only in the graphene interlayer and propose the first ever planar lithium-intercalation model for graphenic carbons. Corroborated by theoretical calculations, various physiochemical characterizations of the staged lithium bilayer graphene products further reveal the regular lithium-intercalation phenomena and thus fully illustrate this elementary lithium storage pattern of two-dimension. These findings not only make the commercial graphite the first electrode with clear lithium-storage process, but also guide the development of graphene materials in lithium ion batteries. More... »

PAGES

275

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-07942-z

DOI

http://dx.doi.org/10.1038/s41467-018-07942-z

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111375450

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30655526


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