Room-temperature electrochemical water–gas shift reaction for high purity hydrogen production View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Xiaoju Cui, Hai-Yan Su, Ruixue Chen, Liang Yu, Jinchao Dong, Chao Ma, Suheng Wang, Jianfeng Li, Fan Yang, Jianping Xiao, Mengtao Zhang, Ding Ma, Dehui Deng, Dong H. Zhang, Zhongqun Tian, Xinhe Bao

ABSTRACT

Traditional water-gas shift reaction provides one primary route for industrial production of clean-energy hydrogen. However, this process operates at high temperatures and pressures, and requires additional separation of H2 from products containing CO2, CH4 and residual CO. Herein, we report a room-temperature electrochemical water-gas shift process for direct production of high purity hydrogen (over 99.99%) with a faradaic efficiency of approximately 100%. Through rational design of anode structure to facilitate CO diffusion and PtCu catalyst to optimize CO adsorption, the anodic onset potential is lowered to almost 0 volts versus the reversible hydrogen electrode at room temperature and atmospheric pressure. The optimized PtCu catalyst achieves a current density of 70.0 mA cm-2 at 0.6 volts which is over 12 times that of commercial Pt/C (40 wt.%) catalyst, and remains stable for even more than 475 h. This study opens a new and promising route of producing high purity hydrogen. More... »

PAGES

86

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-07937-w

DOI

http://dx.doi.org/10.1038/s41467-018-07937-w

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111061197

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30622261


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282 https://www.grid.ac/institutes/grid.12955.3a schema:alternateName Xiamen University
283 schema:name Collaborative Innovation Center of Chemistry for Energy Materials, College of Chemistry and Chemical Engineering, Xiamen University, 361005, Xiamen, China
284 State Key Laboratory of Catalysis, Collaborative Innovation Center of Chemistry for Energy Materials, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 116023, Dalian, China
285 rdf:type schema:Organization
286 https://www.grid.ac/institutes/grid.423905.9 schema:alternateName Dalian Institute of Chemical Physics
287 schema:name State Key Laboratory of Catalysis, Collaborative Innovation Center of Chemistry for Energy Materials, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 116023, Dalian, China
288 State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 116023, Dalian, China
289 rdf:type schema:Organization
290 https://www.grid.ac/institutes/grid.67293.39 schema:alternateName Hunan University
291 schema:name Center for High Resolution Electron Microscopy, College of Materials Science and Engineering, Hunan University, 410082, Changsha, China
292 rdf:type schema:Organization
 




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