Unravelling the effect of charge dynamics at the plasmonic metal/semiconductor interface for CO2 photoreduction View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Laura Collado, Anna Reynal, Fernando Fresno, Mariam Barawi, Carlos Escudero, Virginia Perez-Dieste, Juan M. Coronado, David P. Serrano, James R. Durrant, Víctor A. de la Peña O’Shea

ABSTRACT

Sunlight plays a critical role in the development of emerging sustainable energy conversion and storage technologies. Light-induced CO2 reduction by artificial photosynthesis is one of the cornerstones to produce renewable fuels and environmentally friendly chemicals. Interface interactions between plasmonic metal nanoparticles and semiconductors exhibit improved photoactivities under a wide range of the solar spectrum. However, the photo-induced charge transfer processes and their influence on photocatalysis with these materials are still under debate, mainly due to the complexity of the involved routes occurring at different timescales. Here, we use a combination of advanced in situ and time-resolved spectroscopies covering different timescales, combined with theoretical calculations, to unravel the overall mechanism of photocatalytic CO2 reduction by Ag/TiO2 catalysts. Our findings provide evidence of the key factors determining the enhancement of photoactivity under ultraviolet and visible irradiation, which have important implications for the design of solar energy conversion materials. More... »

PAGES

4986

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-07397-2

DOI

http://dx.doi.org/10.1038/s41467-018-07397-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1110065931

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30478316


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