Stability and nature of the volume collapse of ε-Fe2O3 under extreme conditions View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

J. A. Sans, V. Monteseguro, G. Garbarino, M. Gich, V. Cerantola, V. Cuartero, M. Monte, T. Irifune, A. Muñoz, C. Popescu

ABSTRACT

Iron oxides are among the major constituents of the deep Earth's interior. Among them, the epsilon phase of Fe2O3 is one of the less studied polymorphs and there is a lack of information about its structural, electronic and magnetic transformations at extreme conditions. Here we report the precise determination of its equation of state and a deep analysis of the evolution of the polyhedral units under compression, thanks to the agreement between our experiments and ab-initio simulations. Our results indicate that this material, with remarkable magnetic properties, is stable at pressures up to 27 GPa. Above 27 GPa, a volume collapse has been observed and ascribed to a change of the local environment of the tetrahedrally coordinated iron towards an octahedral coordination, finding evidence for a different iron oxide polymorph. More... »

PAGES

4554

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-06966-9

DOI

http://dx.doi.org/10.1038/s41467-018-06966-9

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1107871602

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30385756


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