Polymerization driven monomer passage through monolayer chemical vapour deposition graphene View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Tao Zhang, Zhongquan Liao, Leonardo Medrano Sandonas, Arezoo Dianat, Xiaoling Liu, Peng Xiao, Ihsan Amin, Rafael Gutierrez, Tao Chen, Ehrenfried Zschech, Gianaurelio Cuniberti, Rainer Jordan

ABSTRACT

Mass transport through graphene is receiving increasing attention due to the potential for molecular sieving. Experimental studies are mostly limited to the translocation of protons, ions, and water molecules, and results for larger molecules through graphene are rare. Here, we perform controlled radical polymerization with surface-anchored self-assembled initiator monolayer in a monomer solution with single-layer graphene separating the initiator from the monomer. We demonstrate that neutral monomers are able to pass through the graphene (via native defects) and increase the graphene defects ratio (Raman ID/IG) from ca. 0.09 to 0.22. The translocations of anionic and cationic monomers through graphene are significantly slower due to chemical interactions of monomers with the graphene defects. Interestingly, if micropatterned initiator-monolayers are used, the translocations of anionic monomers apparently cut the graphene sheet into congruent microscopic structures. The varied interactions between monomers and graphene defects are further investigated by quantum molecular dynamics simulations. More... »

PAGES

4051

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-06599-y

DOI

http://dx.doi.org/10.1038/s41467-018-06599-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1107275376

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30282989


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285 https://www.grid.ac/institutes/grid.4488.0 schema:alternateName TU Dresden
286 schema:name Center for Advancing Electronics Dresden, Technische Universität Dresden, 01062, Dresden, Germany
287 Chair of Macromolecular Chemistry, Faculty of Chemistry and Food Chemistry, School of Science, Technische Universität Dresden, Mommsenstr. 4, 01062, Dresden, Germany
288 Dresden Center for Computational Materials Science, Technische Universität Dresden, 01062, Dresden, Germany
289 Institute for Materials Science and Max Bergmann Center of Biomaterials, Technische Universität Dresden, 01062, Dresden, Germany
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291 https://www.grid.ac/institutes/grid.461622.5 schema:alternateName Fraunhofer Institute for Ceramic Technologies and Systems
292 schema:name Center for Advancing Electronics Dresden, Technische Universität Dresden, 01062, Dresden, Germany
293 Fraunhofer Institute for Ceramic Technologies and Systems (IKTS), Maria-Reiche-Straße 2, 01109, Dresden, Germany
294 Institute for Materials Science and Max Bergmann Center of Biomaterials, Technische Universität Dresden, 01062, Dresden, Germany
295 rdf:type schema:Organization
296 https://www.grid.ac/institutes/grid.461720.6 schema:alternateName Leib­niz In­sti­tu­te for Plas­ma Sci­ence and Tech­no­lo­gy
297 schema:name Chair of Macromolecular Chemistry, Faculty of Chemistry and Food Chemistry, School of Science, Technische Universität Dresden, Mommsenstr. 4, 01062, Dresden, Germany
298 Junior Research Group Biosensing Surfaces, Leibniz Institute for Plasma Science and Technology, INP Greifswald e.V., Felix-Hausdorff-Strasse 2, 17489, Greifswald, Germany
299 rdf:type schema:Organization
300 https://www.grid.ac/institutes/grid.9227.e schema:alternateName Chinese Academy of Sciences
301 schema:name Key Laboratory of Marine Materials and Related Technologies, Zhejiang Key Laboratory of Marine Materials and Protective Technologies, Ningbo Institute of Material Technology and Engineering, Chinese Academy of Sciences, 315201, Ningbo, China
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