An interstellar synthesis of phosphorus oxoacids View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Andrew M. Turner, Alexandre Bergantini, Matthew J. Abplanalp, Cheng Zhu, Sándor Góbi, Bing-Jian Sun, Kang-Heng Chao, Agnes H. H. Chang, Cornelia Meinert, Ralf I. Kaiser

ABSTRACT

Phosphorus signifies an essential element in molecular biology, yet given the limited solubility of phosphates on early Earth, alternative sources like meteoritic phosphides have been proposed to incorporate phosphorus into biomolecules under prebiotic terrestrial conditions. Here, we report on a previously overlooked source of prebiotic phosphorus from interstellar phosphine (PH3) that produces key phosphorus oxoacids-phosphoric acid (H3PO4), phosphonic acid (H3PO3), and pyrophosphoric acid (H4P2O7)-in interstellar analog ices exposed to ionizing radiation at temperatures as low as 5 K. Since the processed material of molecular clouds eventually enters circumstellar disks and is partially incorporated into planetesimals like proto Earth, an understanding of the facile synthesis of oxoacids is essential to untangle the origin of water-soluble prebiotic phosphorus compounds and how they might have been incorporated into organisms not only on Earth, but potentially in our universe as well. More... »

PAGES

3851

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-06415-7

DOI

http://dx.doi.org/10.1038/s41467-018-06415-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1107062179

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30242164


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