Chemisorption of polysulfides through redox reactions with organic molecules for lithium–sulfur batteries View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Ge Li, Xiaolei Wang, Min Ho Seo, Matthew Li, Lu Ma, Yifei Yuan, Tianpin Wu, Aiping Yu, Shun Wang, Jun Lu, Zhongwei Chen

ABSTRACT

Lithium-sulfur battery possesses high energy density but suffers from severe capacity fading due to the dissolution of lithium polysulfides. Novel design and mechanisms to encapsulate lithium polysulfides are greatly desired by high-performance lithium-sulfur batteries towards practical applications. Herein, we report a strategy of utilizing anthraquinone, a natural abundant organic molecule, to suppress dissolution and diffusion of polysulfides species through redox reactions during cycling. The keto groups of anthraquinone play a critical role in forming strong Lewis acid-based chemical bonding. This mechanism leads to a long cycling stability of sulfur-based electrodes. With a high sulfur content of ~73%, a low capacity decay of 0.019% per cycle for 300 cycles and retention of 81.7% over 500 cycles at 0.5 C rate can be achieved. This finding and understanding paves an alternative avenue for the future design of sulfur-based cathodes toward the practical application of lithium-sulfur batteries. More... »

PAGES

705

References to SciGraph publications

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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41467-018-03116-z

    DOI

    http://dx.doi.org/10.1038/s41467-018-03116-z

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1101008467

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/29453414


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