Evolving affinity between Coulombic reversibility and hysteretic phase transformations in nano-structured silicon-based lithium-ion batteries View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

K Ogata, S Jeon, D-S Ko, I S Jung, J H Kim, K Ito, Y Kubo, K Takei, S Saito, Y-H Cho, H Park, J Jang, H-G Kim, J-H Kim, Y S Kim, W Choi, M Koh, K Uosaki, S G Doo, Y Hwang, S Han

ABSTRACT

Nano-structured silicon is an attractive alternative anode material to conventional graphite in lithium-ion batteries. However, the anode designs with higher silicon concentrations remain to be commercialized despite recent remarkable progress. One of the most critical issues is the fundamental understanding of the lithium-silicon Coulombic efficiency. Particularly, this is the key to resolve subtle yet accumulatively significant alterations of Coulombic efficiency by various paths of lithium-silicon processes over cycles. Here, we provide quantitative and qualitative insight into how the irreversible behaviors are altered by the processes under amorphous volume changes and hysteretic amorphous-crystalline phase transformations. Repeated latter transformations over cycles, typically featured as a degradation factor, can govern the reversibility behaviors, improving the irreversibility and eventually minimizing cumulative irreversible lithium consumption. This is clearly different from repeated amorphous volume changes with different lithiation depths. The mechanism behind the correlations is elucidated by electrochemical and structural probing. More... »

PAGES

479

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-018-02824-w

DOI

http://dx.doi.org/10.1038/s41467-018-02824-w

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1100699146

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29396479


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