Caging tin oxide in three-dimensional graphene networks for superior volumetric lithium storage View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Junwei Han, Debin Kong, Wei Lv, Dai-Ming Tang, Daliang Han, Chao Zhang, Donghai Liu, Zhichang Xiao, Xinghao Zhang, Jing Xiao, Xinzi He, Feng-Chun Hsia, Chen Zhang, Ying Tao, Dmitri Golberg, Feiyu Kang, Linjie Zhi, Quan-Hong Yang

ABSTRACT

Tin and its compounds hold promise for the development of high-capacity anode materials that could replace graphitic carbon used in current lithium-ion batteries. However, the introduced porosity in current electrode designs to buffer the volume changes of active materials during cycling does not afford high volumetric performance. Here, we show a strategy leveraging a sulfur sacrificial agent for controlled utility of void space in a tin oxide/graphene composite anode. In a typical synthesis using the capillary drying of graphene hydrogels, sulfur is employed with hard tin oxide nanoparticles inside the contraction hydrogels. The resultant graphene-caged tin oxide delivers an ultrahigh volumetric capacity of 2123 mAh cm-3 together with good cycling stability. Our results suggest not only a conversion-type composite anode that allows for good electrochemical characteristics, but also a general synthetic means to engineering the packing density of graphene nanosheets for high energy storage capabilities in small volumes. More... »

PAGES

402

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-017-02808-2

DOI

http://dx.doi.org/10.1038/s41467-017-02808-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1100570902

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29374156


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