Magnetostriction-polarization coupling in multiferroic Mn2MnWO6 View Full Text


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Article Info

DATE

2017-12-11

AUTHORS

Man-Rong Li, Emma E. McCabe, Peter W. Stephens, Mark Croft, Liam Collins, Sergei V. Kalinin, Zheng Deng, Maria Retuerto, Arnab Sen Gupta, Haricharan Padmanabhan, Venkatraman Gopalan, Christoph P. Grams, Joachim Hemberger, Fabio Orlandi, Pascal Manuel, Wen-Min Li, Chang-Qing Jin, David Walker, Martha Greenblatt

ABSTRACT

Double corundum-related polar magnets are promising materials for multiferroic and magnetoelectric applications in spintronics. However, their design and synthesis is a challenge, and magnetoelectric coupling has only been observed in Ni3TeO6 among the known double corundum compounds to date. Here we address the high-pressure synthesis of a new polar and antiferromagnetic corundum derivative Mn2MnWO6, which adopts the Ni3TeO6-type structure with low temperature first-order field-induced metamagnetic phase transitions (TN = 58 K) and high spontaneous polarization (~ 63.3 μC·cm−2). The magnetostriction-polarization coupling in Mn2MnWO6 is evidenced by second harmonic generation effect, and corroborated by magnetic-field-dependent pyroresponse behavior, which together with the magnetic-field-dependent polarization and dielectric measurements, qualitatively indicate magnetoelectric coupling. Piezoresponse force microscopy imaging and spectroscopy studies on Mn2MnWO6 show switchable polarization, which motivates further exploration on magnetoelectric effect in single crystal/thin film specimens. More... »

PAGES

2037

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-017-02003-3

DOI

http://dx.doi.org/10.1038/s41467-017-02003-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1099597583

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29229914


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19 behavior
20 challenges
21 compounds
22 coupling
23 date
24 dependent polarization
25 design
26 dielectric measurements
27 effect
28 exploration
29 field-induced metamagnetic phase transition
30 film specimens
31 force microscopy imaging
32 further exploration
33 generation effect
34 harmonic generation effect
35 high spontaneous polarization
36 high-pressure synthesis
37 imaging
38 magnetoelectric applications
39 magnetoelectric coupling
40 magnetoelectric effect
41 magnets
42 materials
43 measurements
44 metamagnetic phase transition
45 microscopy imaging
46 multiferroics
47 phase transition
48 piezoresponse force microscopy imaging
49 polar magnets
50 polarization
51 second harmonic generation effect
52 specimens
53 spectroscopy studies
54 spintronics
55 spontaneous polarization
56 structure
57 study
58 switchable polarization
59 synthesis
60 thin film specimens
61 transition
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