Engineering the internal surfaces of three-dimensional nanoporous catalysts by surfactant-modified dealloying View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2017-10-20

AUTHORS

Zhili Wang, Pan Liu, Jiuhui Han, Chun Cheng, Shoucong Ning, Akihiko Hirata, Takeshi Fujita, Mingwei Chen

ABSTRACT

Tuning surface structures by bottom-up synthesis has been demonstrated as an effective strategy to improve the catalytic performances of nanoparticle catalysts. Nevertheless, the surface modification of three-dimensional nanoporous metals, fabricated by a top-down dealloying approach, has not been achieved despite great efforts devoted to improving the catalytic performance of three-dimensional nanoporous catalysts. Here we report a surfactant-modified dealloying method to tailor the surface structure of nanoporous gold for amplified electrocatalysis toward methanol oxidation and oxygen reduction reactions. With the assistance of surfactants, {111} or {100} faceted internal surfaces of nanoporous gold can be realized in a controllable manner by optimizing dealloying conditions. The surface modified nanoporous gold exhibits significantly enhanced electrocatalytic activities in comparison with conventional nanoporous gold. This study paves the way to develop high-performance three-dimensional nanoporous catalysts with a tunable surface structure by top-down dealloying for efficient chemical and electrochemical reactions. More... »

PAGES

1066

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41467-017-01085-3

DOI

http://dx.doi.org/10.1038/s41467-017-01085-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1092252206

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29057916


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