Synthesis of novel nucleobase-terminated organosilane and its self-assembly on a substrate View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2012-06

AUTHORS

Takashi Miyata, Akifumi Kawamura, Terumi Meotoiwa, Moritoshi Matsumoto, Tadashi Uragami

ABSTRACT

A novel nucleobase-terminated organosilane with nucleobase and ethoxysilane moieties was synthesized by a simple method in which bromouracil reacts with amino-terminated organosilane without solvents. The uracil-terminated organosilane was self-assembled on a hydroxylated surface, and then the uracil-concentrated surface was obtained. The resulting uracil-terminated self-assembled layers were characterized by X-ray photoelectron spectroscopy and ellipsometry. Adenine complementary to uracil was effectively adsorbed onto the resultant uracil-concentrated surface by multiple hydrogen bonds. Herein, a simple method is provided for synthesizing a nucleobase-terminated organosilane and modifying a hydroxylated surface to a nucleobase-concentrated surface. Our method, which uses the self-assembly of nucleobase-terminated organosilanes, facilitates the construction of bioconjugated devices for separating and sensing nucleobases and nucleic acids. More... »

PAGES

625

Journal

TITLE

Polymer Journal

ISSUE

6

VOLUME

44

Author Affiliations

From Grant

  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/pj.2012.41

    DOI

    http://dx.doi.org/10.1038/pj.2012.41

    DIMENSIONS

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