Non-equilibrium singlet–triplet Kondo effect in carbon nanotubes View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2006-07

AUTHORS

J. Paaske, A. Rosch, P. Wölfle, N. Mason, C. M. Marcus, J. Nygård

ABSTRACT

The Kondo effect is a many-body phenomenon arising due to conduction electrons scattering off a localized spin1. Coherent spin-flip scattering off such a quantum impurity correlates the conduction electrons, and at low temperature this leads to a zero-bias conductance anomaly2,3. This has become a common signature in bias spectroscopy of single-electron transistors, observed in GaAs quantum dots4,5,6,7,8,9 as well as in various single-molecule transistors10,11,12,13,14,15. Although the zero-bias Kondo effect is well established, the extent to which Kondo correlations persist in non-equilibrium situations where inelastic processes induce decoherence remains uncertain. Here we report on a pronounced conductance peak observed at finite bias voltage in a carbon-nanotube quantum dot in the spin-singlet ground state. We explain this finite-bias conductance anomaly by a non-equilibrium Kondo effect involving excitations into a spin-triplet state. Excellent agreement between calculated and measured nonlinear conductance is obtained, thus strongly supporting the correlated nature of this non-equilibrium resonance. More... »

PAGES

460-464

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nphys340

DOI

http://dx.doi.org/10.1038/nphys340

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1007824539


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32 schema:description The Kondo effect is a many-body phenomenon arising due to conduction electrons scattering off a localized spin1. Coherent spin-flip scattering off such a quantum impurity correlates the conduction electrons, and at low temperature this leads to a zero-bias conductance anomaly2,3. This has become a common signature in bias spectroscopy of single-electron transistors, observed in GaAs quantum dots4,5,6,7,8,9 as well as in various single-molecule transistors10,11,12,13,14,15. Although the zero-bias Kondo effect is well established, the extent to which Kondo correlations persist in non-equilibrium situations where inelastic processes induce decoherence remains uncertain. Here we report on a pronounced conductance peak observed at finite bias voltage in a carbon-nanotube quantum dot in the spin-singlet ground state. We explain this finite-bias conductance anomaly by a non-equilibrium Kondo effect involving excitations into a spin-triplet state. Excellent agreement between calculated and measured nonlinear conductance is obtained, thus strongly supporting the correlated nature of this non-equilibrium resonance.
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