Thermal activation of non-radiative Auger recombination in charged colloidal nanocrystals View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2013-03

AUTHORS

C. Javaux, B. Mahler, B. Dubertret, A. Shabaev, A. V. Rodina, Al. L. Efros, D. R. Yakovlev, F. Liu, M. Bayer, G. Camps, L. Biadala, S. Buil, X. Quelin, J-P. Hermier

ABSTRACT

Applications of semiconductor nanocrystals such as biomarkers and light-emitting optoelectronic devices require that their fluorescence quantum yield be close to 100%. However, such quantum yields have not been obtained yet, in part, because non-radiative Auger recombination in charged nanocrystals could not be suppressed completely. Here, we synthesize colloidal core/thick-shell CdSe/CdS nanocrystals with 100% quantum yield and completely quenched Auger processes at low temperatures, although the nanocrystals are negatively photocharged. Single particle and ensemble spectroscopy in the temperature range 30-300 K shows that the non-radiative Auger recombination is thermally activated around 200 K. Experimental results are well described by a model suggesting a temperature-dependent delocalization of one of the trion electrons from the CdSe core and enhanced Auger recombination at the abrupt CdS outer surface. These results point to a route for the design of core/shell structures with 100% quantum yield at room temperature. More... »

PAGES

206

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nnano.2012.260

DOI

http://dx.doi.org/10.1038/nnano.2012.260

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1018977568

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23396313


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