Nanopatterning self-assembled nanoparticle superlattices by moulding microdroplets View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2008-11

AUTHORS

Wenlong Cheng, Nokyoung Park, M Todd Walter, Mark R Hartman, Dan Luo

ABSTRACT

Highly ordered arrays of nanoparticles exhibit many properties that are not found in their disordered counterparts. However, these nanoparticle superlattices usually form in a far-from-equilibrium dewetting process, which precludes the use of conventional patterning methods owing to a lack of control over the local dewetting dynamics. Here, we report a simple yet efficient approach for patterning such superlattices that involves moulding microdroplets containing the nanoparticles and spatially regulating their dewetting process. This approach can provide rational control over the local nucleation and growth of the nanoparticle superlattices. Using DNA-capped gold nanoparticles as a model system, we have patterned nanoparticle superlattices over large areas into a number of versatile structures with high degrees of internal order, including single-particle-width corrals, single-particle-thickness microdiscs and submicrometre-sized 'supra-crystals'. Remarkably, these features could be addressed by micropatterned electrode arrays, suggesting potential applications in bottom-up nanodevices. More... »

PAGES

682-690

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nnano.2008.279

DOI

http://dx.doi.org/10.1038/nnano.2008.279

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1026126509

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/18989335


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