Safe and recyclable lithium-ion capacitors using sacrificial organic lithium salt View Full Text


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Article Info

DATE

2018-02

AUTHORS

P. Jeżowski, O. Crosnier, E. Deunf, P. Poizot, F. Béguin, T. Brousse

ABSTRACT

Lithium-ion capacitors (LICs) shrewdly combine a lithium-ion battery negative electrode capable of reversibly intercalating lithium cations, namely graphite, together with an electrical double-layer positive electrode, namely activated carbon. However, the beauty of this concept is marred by the lack of a lithium-cation source in the device, thus requiring a specific preliminary charging step. The strategies devised thus far in an attempt to rectify this issue all present drawbacks. Our research uncovers a unique approach based on the use of a lithiated organic material, namely 3,4-dihydroxybenzonitrile dilithium salt. This compound can irreversibly provide lithium cations to the graphite electrode during an initial operando charging step without any negative effects with respect to further operation of the LIC. This method not only restores the low CO2 footprint of LICs, but also possesses far-reaching potential with respect to designing a wide range of greener hybrid devices based on other chemistries, comprising entirely recyclable components. More... »

PAGES

167

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nmat5029

DOI

http://dx.doi.org/10.1038/nmat5029

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1099638485

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29251724


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