Origin of voltage decay in high-capacity layered oxide electrodes View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2015-02

AUTHORS

M Sathiya, A M Abakumov, D Foix, G Rousse, K Ramesha, M Saubanère, M L Doublet, H Vezin, C P Laisa, A S Prakash, D Gonbeau, G VanTendeloo, J-M Tarascon

ABSTRACT

Although Li-rich layered oxides (Li1+xNiyCozMn1-x-y-zO2 > 250 mAh g(-1)) are attractive electrode materials providing energy densities more than 15% higher than today's commercial Li-ion cells, they suffer from voltage decay on cycling. To elucidate the origin of this phenomenon, we employ chemical substitution in structurally related Li2RuO3 compounds. Li-rich layered Li2Ru1-yTiyO3 phases with capacities of ~240 mAh g(-1) exhibit the characteristic voltage decay on cycling. A combination of transmission electron microscopy and X-ray photoelectron spectroscopy studies reveals that the migration of cations between metal layers and Li layers is an intrinsic feature of the charge-discharge process that increases the trapping of metal ions in interstitial tetrahedral sites. A correlation between these trapped ions and the voltage decay is established by expanding the study to both Li2Ru1-ySnyO3 and Li2RuO3; the slowest decay occurs for the cations with the largest ionic radii. This effect is robust, and the finding provides insights into new chemistry to be explored for developing high-capacity layered electrodes that evade voltage decay. More... »

PAGES

230-238

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nmat4137

DOI

http://dx.doi.org/10.1038/nmat4137

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1032548579

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25437258


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