Speed limit of the insulator–metal transition in magnetite View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-10

AUTHORS

S. de Jong, R. Kukreja, C. Trabant, N. Pontius, C. F. Chang, T. Kachel, M. Beye, F. Sorgenfrei, C. H. Back, B. Bräuer, W. F. Schlotter, J. J. Turner, O. Krupin, M. Doehler, D. Zhu, M. A. Hossain, A. O. Scherz, D. Fausti, F. Novelli, M. Esposito, W. S. Lee, Y. D. Chuang, D. H. Lu, R. G. Moore, M. Yi, M. Trigo, P. Kirchmann, L. Pathey, M. S. Golden, M. Buchholz, P. Metcalf, F. Parmigiani, W. Wurth, A. Föhlisch, C. Schüßler-Langeheine, H. A. Dürr

ABSTRACT

As the oldest known magnetic material, magnetite (Fe3O4) has fascinated mankind for millennia. As the first oxide in which a relationship between electrical conductivity and fluctuating/localized electronic order was shown, magnetite represents a model system for understanding correlated oxides in general. Nevertheless, the exact mechanism of the insulator-metal, or Verwey, transition has long remained inaccessible. Recently, three-Fe-site lattice distortions called trimerons were identified as the characteristic building blocks of the low-temperature insulating electronically ordered phase. Here we investigate the Verwey transition with pump-probe X-ray diffraction and optical reflectivity techniques, and show how trimerons become mobile across the insulator-metal transition. We find this to be a two-step process. After an initial 300 fs destruction of individual trimerons, phase separation occurs on a 1.5±0.2 ps timescale to yield residual insulating and metallic regions. This work establishes the speed limit for switching in future oxide electronics. More... »

PAGES

882

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nmat3718

DOI

http://dx.doi.org/10.1038/nmat3718

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1013280874

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23892787


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432 https://www.grid.ac/institutes/grid.5942.a schema:alternateName Elettra Sincrotrone Trieste
433 schema:name Department of Physics, University of Trieste, 34127 Trieste, Italy
434 Elettra-Sincrotrone Trieste SCnA, Basovizza I-34012, Italy
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436 https://www.grid.ac/institutes/grid.5991.4 schema:alternateName Paul Scherrer Institute
437 schema:name SwissFEL, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland
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439 https://www.grid.ac/institutes/grid.6190.e schema:alternateName University of Cologne
440 schema:name Universität zu Köln, II. Physikalisches Institut, Zülpicher Straße 77, 50937 Köln, Germany
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442 https://www.grid.ac/institutes/grid.7177.6 schema:alternateName University of Amsterdam
443 schema:name Stanford Institute for Energy and Materials Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
444 Van der Waals-Zeeman Institute, University of Amsterdam, Science Park 904, 1098 XH Amsterdam, The Netherlands
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446 https://www.grid.ac/institutes/grid.7727.5 schema:alternateName University of Regensburg
447 schema:name Stanford Institute for Energy and Materials Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
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450 https://www.grid.ac/institutes/grid.9026.d schema:alternateName University of Hamburg
451 schema:name Helmholtz-Zentrum Berlin für Materialien und Energie, Albert-Einstein-Str. 15, 12489 Berlin, Germany
452 Universität Hamburg, Department of Physics and Center for Free-Electron Laser Science, Luruper Chaussee 149, 22761 Hamburg, Germany
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