Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-09

AUTHORS

Damien Voiry, Hisato Yamaguchi, Junwen Li, Rafael Silva, Diego C. B. Alves, Takeshi Fujita, Mingwei Chen, Tewodros Asefa, Vivek B. Shenoy, Goki Eda, Manish Chhowalla

ABSTRACT

Efficient evolution of hydrogen through electrocatalysis at low overpotentials holds tremendous promise for clean energy. Hydrogen evolution can be easily achieved by electrolysis at large potentials that can be lowered with expensive platinum-based catalysts. Replacement of Pt with inexpensive, earth-abundant electrocatalysts would be significantly beneficial for clean and efficient hydrogen evolution. To this end, promising results have been reported using 2H (trigonal prismatic) XS₂ (where X = Mo or W) nanoparticles with a high concentration of metallic edges. The key challenges for XS₂ are increasing the number and catalytic activity of active sites. Here we report monolayered nanosheets of chemically exfoliated WS₂ as efficient catalysts for hydrogen evolution with very low overpotentials. Analyses indicate that the enhanced electrocatalytic activity of WS₂ is associated with the high concentration of the strained metallic 1T (octahedral) phase in the as-exfoliated nanosheets. Our results suggest that chemically exfoliated WS₂ nanosheets are interesting catalysts for hydrogen evolution. More... »

PAGES

850

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nmat3700

DOI

http://dx.doi.org/10.1038/nmat3700

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1048205566

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23832127


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