Catalytically highly active top gold atom on palladium nanocluster View Full Text


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Article Info

DATE

2012-01

AUTHORS

Haijun Zhang, Tatsuya Watanabe, Mitsutaka Okumura, Masatake Haruta, Naoki Toshima

ABSTRACT

Catalysis using gold is emerging as an important field of research in connection with 'green' chemistry. Several hypotheses have been presented to explain the markedly high activities of Au catalysts. So far, the origin of the catalytic activities of supported Au catalysts can be assigned to the perimeter interfaces between Au nanoclusters and the support. However, the genesis of the catalytic activities of colloidal Au-based bimetallic nanoclusters is unclear. Moreover, it is still a challenge to synthesize Au-based colloidal catalysts with high activity. Here we now present the 'crown-jewel' concept (Supplementary Fig. S1) for preparation of catalytically highly Au-based colloidal catalysts. Au-Pd colloidal catalysts containing an abundance of top (vertex or corner) Au atoms were synthesized according to the strategy on a large scale. Our results indicate that the genesis of the high activity of the catalysts could be ascribed to the presence of negatively charged top Au atoms. More... »

PAGES

49

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nmat3143

DOI

http://dx.doi.org/10.1038/nmat3143

DIMENSIONS

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PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/22019941


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