Large-area synthesis of high-quality and uniform monolayer WS2 on reusable Au foils View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-12

AUTHORS

Yang Gao, Zhibo Liu, Dong-Ming Sun, Le Huang, Lai-Peng Ma, Li-Chang Yin, Teng Ma, Zhiyong Zhang, Xiu-Liang Ma, Lian-Mao Peng, Hui-Ming Cheng, Wencai Ren

ABSTRACT

Large-area monolayer WS2 is a desirable material for applications in next-generation electronics and optoelectronics. However, the chemical vapour deposition (CVD) with rigid and inert substrates for large-area sample growth suffers from a non-uniform number of layers, small domain size and many defects, and is not compatible with the fabrication process of flexible devices. Here we report the self-limited catalytic surface growth of uniform monolayer WS2 single crystals of millimetre size and large-area films by ambient-pressure CVD on Au. The weak interaction between the WS2 and Au enables the intact transfer of the monolayers to arbitrary substrates using the electrochemical bubbling method without sacrificing Au. The WS2 shows high crystal quality and optical and electrical properties comparable or superior to mechanically exfoliated samples. We also demonstrate the roll-to-roll/bubbling production of large-area flexible films of uniform monolayer, double-layer WS2 and WS2/graphene heterostructures, and batch fabrication of large-area flexible monolayer WS2 film transistor arrays. More... »

PAGES

8569

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms9569

DOI

http://dx.doi.org/10.1038/ncomms9569

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1000825055

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26450174


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