Na+ intercalation pseudocapacitance in graphene-coupled titanium oxide enabling ultra-fast sodium storage and long-term cycling View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-12

AUTHORS

Chaoji Chen, Yanwei Wen, Xianluo Hu, Xiulei Ji, Mengyu Yan, Liqiang Mai, Pei Hu, Bin Shan, Yunhui Huang

ABSTRACT

Sodium-ion batteries are emerging as a highly promising technology for large-scale energy storage applications. However, it remains a significant challenge to develop an anode with superior long-term cycling stability and high-rate capability. Here we demonstrate that the Na(+) intercalation pseudocapacitance in TiO2/graphene nanocomposites enables high-rate capability and long cycle life in a sodium-ion battery. This hybrid electrode exhibits a specific capacity of above 90 mA h g(-1) at 12,000 mA g(-1) (∼36 C). The capacity is highly reversible for more than 4,000 cycles, the longest demonstrated cyclability to date. First-principle calculations demonstrate that the intimate integration of graphene with TiO2 reduces the diffusion energy barrier, thus enhancing the Na(+) intercalation pseudocapacitive process. The Na-ion intercalation pseudocapacitance enabled by tailor-deigned nanostructures represents a promising strategy for developing electrode materials with high power density and long cycle life. More... »

PAGES

6929

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms7929

DOI

http://dx.doi.org/10.1038/ncomms7929

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1014181475

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25906991


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