Methane hydrate formation in confined nanospace can surpass nature View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-03-02

AUTHORS

Mirian E. Casco, Joaquín Silvestre-Albero, Anibal J. Ramírez-Cuesta, Fernando Rey, Jose L. Jordá, Atul Bansode, Atsushi Urakawa, Inma Peral, Manuel Martínez-Escandell, Katsumi Kaneko, Francisco Rodríguez-Reinoso

ABSTRACT

Natural methane hydrates are believed to be the largest source of hydrocarbons on Earth. These structures are formed in specific locations such as deep-sea sediments and the permafrost based on demanding conditions of high pressure and low temperature. Here we report that, by taking advantage of the confinement effects on nanopore space, synthetic methane hydrates grow under mild conditions (3.5 MPa and 2 °C), with faster kinetics (within minutes) than nature, fully reversibly and with a nominal stoichiometry that mimics nature. The formation of the hydrate structures in nanospace and their similarity to natural hydrates is confirmed using inelastic neutron scattering experiments and synchrotron X-ray powder diffraction. These findings may be a step towards the application of a smart synthesis of methane hydrates in energy-demanding applications (for example, transportation). More... »

PAGES

6432

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms7432

DOI

http://dx.doi.org/10.1038/ncomms7432

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1006825175

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25728378


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