Ultra-sensitive optical oxygen sensors for characterization of nearly anoxic systems View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2014-12

AUTHORS

Philipp Lehner, Christoph Staudinger, Sergey M. Borisov, Ingo Klimant

ABSTRACT

Oxygen quantification in trace amounts is essential in many fields of science and technology. Optical oxygen sensors proved invaluable tools for oxygen measurements in a broad concentration range, but until now neither optical nor electrochemical oxygen sensors were able to quantify oxygen in the sub-nanomolar concentration range. Herein we present new optical oxygen-sensing materials with unmatched sensitivity. They rely on the combination of ultra-long decaying (several 100 ms lifetime) phosphorescent boron- and aluminium-chelates, and highly oxygen-permeable and chemically stable perfluorinated polymers. The sensitivity of the new sensors is improved up to 20-fold compared with state-of-the-art analogues. The limits of detection are as low as 5 p.p.b., volume in gas phase under atmospheric pressure or 7 pM in solution. The sensors enable completely new applications for monitoring of oxygen in previously inaccessible concentration ranges. More... »

PAGES

4460

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms5460

DOI

http://dx.doi.org/10.1038/ncomms5460

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1014808472

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25042041


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