Chiral plasmonic DNA nanostructures with switchable circular dichroism View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-12

AUTHORS

Robert Schreiber, Ngoc Luong, Zhiyuan Fan, Anton Kuzyk, Philipp C. Nickels, Tao Zhang, David M. Smith, Bernard Yurke, Wan Kuang, Alexander O. Govorov, Tim Liedl

ABSTRACT

Circular dichroism spectra of naturally occurring molecules and also of synthetic chiral arrangements of plasmonic particles often exhibit characteristic bisignate shapes. Such spectra consist of peaks next to dips (or vice versa) and result from the superposition of signals originating from many individual chiral objects oriented randomly in solution. Here we show that by first aligning and then toggling the orientation of DNA-origami-scaffolded nanoparticle helices attached to a substrate, we are able to reversibly switch the optical response between two distinct circular dichroism spectra corresponding to either perpendicular or parallel helix orientation with respect to the light beam. The observed directional circular dichroism of our switchable plasmonic material is in good agreement with predictions based on dipole approximation theory. Such dynamic metamaterials introduce functionality into soft matter-based optical devices and may enable novel data storage schemes or signal modulators. More... »

PAGES

2948

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms3948

DOI

http://dx.doi.org/10.1038/ncomms3948

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1026421912

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/24336125


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