Molecular origin of high field-effect mobility in an indacenodithiophene–benzothiadiazole copolymer View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-12

AUTHORS

Xinran Zhang, Hugo Bronstein, Auke J. Kronemeijer, Jeremy Smith, Youngju Kim, R. Joseph Kline, Lee J. Richter, Thomas D. Anthopoulos, Henning Sirringhaus, Kigook Song, Martin Heeney, Weimin Zhang, Iain McCulloch, Dean M. DeLongchamp

ABSTRACT

One of the most inspiring and puzzling developments in the organic electronics community in the last few years has been the emergence of solution-processable semiconducting polymers that lack significant long-range order but outperform the best, high-mobility, ordered semiconducting polymers to date. Here we provide new insights into the charge-transport mechanism in semiconducting polymers and offer new molecular design guidelines by examining a state-of-the-art indacenodithiophene-benzothiadiazole copolymer having field-effect mobility of up to 3.6 cm(2) V(-1) s(-1) with a combination of diffraction and polarizing spectroscopic techniques. Our results reveal that its conjugated planes exhibit a common, comprehensive orientation in both the non-crystalline regions and the ordered crystallites, which is likely to originate from its superior backbone rigidity. We argue that charge transport in high-mobility semiconducting polymers is quasi one-dimensional, that is, predominantly occurring along the backbone, and requires only occasional intermolecular hopping through short π-stacking bridges. More... »

PAGES

2238

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms3238

DOI

http://dx.doi.org/10.1038/ncomms3238

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1026191130

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23900027


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