Assembly and control of 3D nematic dipolar colloidal crystals View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-12

AUTHORS

A. Nych, U. Ognysta, M. Škarabot, M. Ravnik, S. Žumer, I. Muševič

ABSTRACT

Topology has long been considered as an abstract mathematical discipline with little connection to material science. Here we demonstrate that control over spatial and temporal positioning of topological defects allows for the design and assembly of three-dimensional nematic colloidal crystals, giving some unexpected material properties, such as giant electrostriction and collective electro-rotation. Using laser tweezers, we have assembled three-dimensional colloidal crystals made up of 4 μm microspheres in a bulk nematic liquid crystal, implementing a step-by-step protocol, dictated by the orientation of point defects. The three-dimensional colloidal crystals have tetragonal symmetry with antiparallel topological dipoles and exhibit giant electrostriction, shrinking by 25-30% at 0.37 V μm(-1). An external electric field induces a reversible and controllable electro-rotation of the crystal as a whole, with the angle of rotation being ~30° at 0.14 V μm(-1), when using liquid crystal with negative dielectric anisotropy. This demonstrates a new class of electrically highly responsive soft materials. More... »

PAGES

1489

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms2486

DOI

http://dx.doi.org/10.1038/ncomms2486

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1007892269

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23403589


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35 schema:description Topology has long been considered as an abstract mathematical discipline with little connection to material science. Here we demonstrate that control over spatial and temporal positioning of topological defects allows for the design and assembly of three-dimensional nematic colloidal crystals, giving some unexpected material properties, such as giant electrostriction and collective electro-rotation. Using laser tweezers, we have assembled three-dimensional colloidal crystals made up of 4 μm microspheres in a bulk nematic liquid crystal, implementing a step-by-step protocol, dictated by the orientation of point defects. The three-dimensional colloidal crystals have tetragonal symmetry with antiparallel topological dipoles and exhibit giant electrostriction, shrinking by 25-30% at 0.37 V μm(-1). An external electric field induces a reversible and controllable electro-rotation of the crystal as a whole, with the angle of rotation being ~30° at 0.14 V μm(-1), when using liquid crystal with negative dielectric anisotropy. This demonstrates a new class of electrically highly responsive soft materials.
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