Uniform electroactive fibre-like micelle nanowires for organic electronics View Full Text


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Article Info

DATE

2017-06-26

AUTHORS

Xiaoyu Li, Piotr J. Wolanin, Liam R. MacFarlane, Robert L. Harniman, Jieshu Qian, Oliver E. C. Gould, Thomas G. Dane, John Rudin, Martin J. Cryan, Thomas Schmaltz, Holger Frauenrath, Mitchell A. Winnik, Charl F. J. Faul, Ian Manners

ABSTRACT

Micelles formed by the self-assembly of block copolymers in selective solvents have attracted widespread attention and have uses in a wide variety of fields, whereas applications based on their electronic properties are virtually unexplored. Herein we describe studies of solution-processable, low-dispersity, electroactive fibre-like micelles of controlled length from π-conjugated diblock copolymers containing a crystalline regioregular poly(3-hexylthiophene) core and a solubilizing, amorphous regiosymmetric poly(3-hexylthiophene) or polystyrene corona. Tunnelling atomic force microscopy measurements demonstrate that the individual fibres exhibit appreciable conductivity. The fibres were subsequently incorporated as the active layer in field-effect transistors. The resulting charge carrier mobility strongly depends on both the degree of polymerization of the core-forming block and the fibre length, and is independent of corona composition. The use of uniform, colloidally stable electroactive fibre-like micelles based on common π-conjugated block copolymers highlights their significant potential to provide fundamental insight into charge carrier processes in devices, and to enable future electronic applications. More... »

PAGES

15909

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms15909

DOI

http://dx.doi.org/10.1038/ncomms15909

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1086206035

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/28649998


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