Neutral and charged inter-valley biexcitons in monolayer MoSe2 View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2017-06-28

AUTHORS

Kai Hao, Judith F. Specht, Philipp Nagler, Lixiang Xu, Kha Tran, Akshay Singh, Chandriker Kavir Dass, Christian Schüller, Tobias Korn, Marten Richter, Andreas Knorr, Xiaoqin Li, Galan Moody

ABSTRACT

In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of the Coulomb interaction leads to strongly correlated many-body states, including excitons and trions, that dominate the optical properties. Higher-order states, such as bound biexcitons, are possible but are difficult to identify unambiguously using linear optical spectroscopy methods. Here, we implement polarization-resolved two-dimensional coherent spectroscopy (2DCS) to unravel the complex optical response of monolayer MoSe2 and identify multiple higher-order correlated states. Decisive signatures of neutral and charged inter-valley biexcitons appear in cross-polarized two-dimensional spectra as distinct resonances with respective ∼20 and ∼5 meV binding energies-similar to recent calculations using variational and Monte Carlo methods. A theoretical model considering the valley-dependent optical selection rules reveals the quantum pathways that give rise to these states. Inter-valley biexcitons identified here, comprising of neutral and charged excitons from different valleys, offer new opportunities for developing ultrathin biexciton lasers and polarization-entangled photon sources. More... »

PAGES

15552

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms15552

DOI

http://dx.doi.org/10.1038/ncomms15552

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1090275464

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/28656961


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