Magnetodielectric detection of magnetic quadrupole order in Ba(TiO)Cu4(PO4)4 with Cu4O12 square cupolas View Full Text


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Article Info

DATE

2016-10-04

AUTHORS

K. Kimura, P. Babkevich, M. Sera, M. Toyoda, K. Yamauchi, G. S. Tucker, J. Martius, T. Fennell, P. Manuel, D. D. Khalyavin, R. D. Johnson, T. Nakano, Y. Nozue, H. M. Rønnow, T. Kimura

ABSTRACT

In vortex-like spin arrangements, multiple spins can combine into emergent multipole moments. Such multipole moments have broken space-inversion and time-reversal symmetries, and can therefore exhibit linear magnetoelectric (ME) activity. Three types of such multipole moments are known: toroidal; monopole; and quadrupole moments. So far, however, the ME activity of these multipole moments has only been established experimentally for the toroidal moment. Here we propose a magnetic square cupola cluster, in which four corner-sharing square-coordinated metal-ligand fragments form a noncoplanar buckled structure, as a promising structural unit that carries an ME-active multipole moment. We substantiate this idea by observing clear magnetodielectric signals associated with an antiferroic ME-active magnetic quadrupole order in the real material Ba(TiO)Cu4(PO4)4. The present result serves as a useful guide for exploring and designing new ME-active materials based on vortex-like spin arrangements. More... »

PAGES

13039

References to SciGraph publications

  • 2007-12. Infinite-layer iron oxide with a square-planar coordination in NATURE
  • 2003-11-06. Magnetic control of ferroelectric polarization in NATURE
  • 2014-09-05. Ferroic nature of magnetic toroidal order in NATURE COMMUNICATIONS
  • 1998-07. Magnetoelectric effect and toroidal ordering in Ga2−xFexO3 in JOURNAL OF EXPERIMENTAL AND THEORETICAL PHYSICS
  • 2013-06-26. Magnetoelectric control of frozen state in a toroidal glass in NATURE COMMUNICATIONS
  • 2007-10. Observation of ferrotoroidic domains in NATURE
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    http://scigraph.springernature.com/pub.10.1038/ncomms13039

    DOI

    http://dx.doi.org/10.1038/ncomms13039

    DIMENSIONS

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    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/27698426


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